Large Places by Wren Schultz courtesy of Blog du Wren.
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DOWN
1. Plead
2. Goes astray
3. Asian nanny
4. The Luncheon on the Grass painter
5. Often chocolate go-with
6. Military letters letters
7. A pop
8. Noah's ride
9. Copenhagen is its hub
10. Causes a broken circuit, maybe
11. Cash says she's gone
12. Mary-Kate or Ashley
13. Matilda writer Dahl
18. Common garden flower
21. "___ walk through the valley..."
23. Played bottom row in a pyramid
24. Quarantine
25. OJ's judge
26. Stat!
27. Enthralled
28. It may be Yellowfin or Bluefin
32. _____ Housewives
34. Indonesia governs part of it
36. Srs exams
37. Docs orgs
38. Sports Center station
41. _____ Fables
43. Simpsons shopkeep
46. Suggary suffix
48. Getting smarter, with "up"
50. Neighbor of 22 across
51. MPs quarries
52. Superman's real real name
53. Actor's resume
56. Tricky pattern
57. Close or tight follower
59. It is based in SLC
60. Leftover bit
61. Flagstaff sch.
62. Tonic go-with
63. Dolittle and Demento
ACROSS
1. Width of a boat
5. Spanishs munchies
10. Stank
14. Writer Bombeck
15. Aida for example
16. Bicycle pref.
17. LARGE North Dakota place
19. Literary lioness
20. Pre-Box cereal measure
21. Under the sea princess
22. LARGE Hawaii place
26. Oft debated subject
29. Ewes mileaus
30. Juan's uncle
31. Riyad denizen
33. Explorer Hernando de ____
35. Tennis great
39. Sleep _____
40. Lily or Whitney
41. First second in command (and second first)
42. School groups
43. Eve's man
44. Legally end
45. Squirt or surge
47. Bad parkers' punishments
49. W2 info
50. LARGE upper midwest place
54. Onto
55. Baby doctor of note
58. Mardi Gras loc.
59. LARGE New York place
64. French resort town ______ les Bains
65. Clog spot
66. Mejhem ibn Meheid, for one
67. Man or Wight
68. Received hurtful words
69. The Simpsons Barney and others

Solution can be found at http://www.blogduwren.com/crosswords/crossword4_solution.gif.
Printable version can be found here.